Numbers 3:49

Therefore, Moses took the money for those that were in excess, and whom they had redeemed from the Levite

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And Moses took the redemption money of them that were over and above them that were redeemed by the Levites:

So Moses took the redemption money from those who were over and above those redeemed by the Levites.

So Moses collected the redemption money from those who exceeded the number redeemed by the Levites.